Nanodiamond-rich layer across three continents consistent with major cosmic impact at 12,800 cal BP


Por: Kinzie C.R., Hee S.S.Q., Stich A., Tague K.A., Mercer C., Razink J.J., Kennett D.J., DeCarli P.S., Bunch T.E., Wittke J.H., Israde-Alcántara I., Bischoff J.L., Goodyear A.C., Tankersley K.B., Kimbel D.R., Culleton B.J., Erlandson J.M., Stafford T.W., Kloosterman J.B., Moore A.M.T., Firestone R.B., Aura Tortosa J.E., Jordá Pardo J.F., West A., Kennett J.P., Wolbach W.S.

Publicada: 1 ene 2014
Categoría: Geology

Resumen:
A major cosmic-impact event has been proposed at the onset of the Younger Dryas (YD) cooling episode at ≈12,800 ± 150 years before present, forming the YD Boundary (YDB) layer, distributed over 150 million km2 on four continents. In 24 dated stratigraphic sections in 10 countries of the Northern Hemisphere, the YDB layer contains a clearly defined abundance peak in nanodiamonds (NDs), a major cosmic-impact proxy. Observed ND polytypes include cubic diamonds, lonsdaleite-like crystals, and diamond-like carbon nanoparticles, called n-diamond and i-carbon. The ND abundances in bulk YDB sediments ranged up to ≈500 ppb (mean: 200 ppb) and that in carbon spherules up to ≈3700 ppb (mean: ≈750 ppb); 138 of 205 sediment samples (67%) contained no detectable NDs. Isotopic evidence indicates that YDB NDs were produced from terrestrial carbon, as with other impact diamonds, and were not derived from the impactor itself. The YDB layer is also marked by abundance peaks in other impact-related proxies, including cosmic-impact spherules, carbon spherules (some containing NDs), iridium, osmium, platinum, charcoal, aciniform carbon (soot), and high-temperature melt-glass. This contribution reviews the debate about the presence, abundance, and origin of the concentration peak in YDB NDs.We describe an updated protocol for the extraction and concentration of NDs from sediment, carbon spherules, and ice, and we describe the basis for identification and classification of YDB ND polytypes, using nine analytical approaches. The large body of evidence now obtained about YDB NDs is strongly consistent with an origin by cosmic impact at ≈12,800 cal BP and is inconsistent with formation of YDB NDs by natural terrestrial processes, including wildfires, anthropogenesis, and/or influx of cosmic dust. © 2014 by The University of Chicago. All rights reserved.

Filiaciones:
Kinzie C.R.:
 Department of Chemistry, DePaul University, Chicago, IL 60614, United States

Hee S.S.Q.:
 Department of Environmental Health Sciences, UCLA Center for Occupational and Environmental Health, University of California, Los Angeles, CA 90095, United States

Stich A.:
 Department of Chemistry, DePaul University, Chicago, IL 60614, United States

Tague K.A.:
 Department of Chemistry, DePaul University, Chicago, IL 60614, United States

Mercer C.:
 National Institute for Materials Science, Tsukuba, 305-0047, Japan

Razink J.J.:
 Center for Advanced Materials Characterization at Oregon, University of Oregon, Eugene, OR 97403, United States

Kennett D.J.:
 Department of Anthropology, Pennsylvania State University, University Park, PA 16802, United States

DeCarli P.S.:
 SRI International, Menlo Park, CA 94025, United States

Bunch T.E.:
 School of Earth Science and Environmental Sustainability, Northern Arizona University, Flagstaff, AZ 86011, United States

Wittke J.H.:
 School of Earth Science and Environmental Sustainability, Northern Arizona University, Flagstaff, AZ 86011, United States

Israde-Alcántara I.:
 Departamento de Geología y Mineralogía Edificio U-4, Instituto de Ciencias de la Tierra, Universidad Michoacana de San Nicolás de Hidalgo, Morelia, Michoacán C.P. 58060, Mexico

Bischoff J.L.:
 US Geological Survey, Menlo Park, CA 94025, United States

Goodyear A.C.:
 South Carolina Institute of Archaeology and Anthropology, University of South Carolina, Columbia, SC 29208, United States

Tankersley K.B.:
 Departments of Anthropology and Geology, University of Cincinnati, Cincinnati, OH 45221, United States

Kimbel D.R.:
 Kimstar Research, Fayetteville, NC 28312, United States

Culleton B.J.:
 Department of Anthropology, Pennsylvania State University, University Park, PA 16802, United States

Erlandson J.M.:
 Museum of Natural and Cultural History, University of Oregon, Eugene, OR 97403, United States

Stafford T.W.:
 AMS 14 C Dating Centre, Department of Physics and Astronomy, University of Aarhus, Ny Munkegade 120Aarhus, Denmark

 Centre for GeoGenetics, Natural History Museum of Denmark, Geological Museum, Oester Voldgade 5-7, Copenhagen, DK-1350, Denmark

Kloosterman J.B.:
 Exploration Geologist, Amsterdam, 1016NN, Netherlands

Moore A.M.T.:
 College of Liberal Arts, Rochester Institute of Technology, Rochester, NY 14623, United States

Firestone R.B.:
 Lawrence Berkeley National Laboratory, Berkeley, CA 94720, United States

Aura Tortosa J.E.:
 Departament de Prehistòria i Arqueologia, Universitat de València, Avenida Blasco Ibáñez 28, Valencia, E-46010, Spain

Jordá Pardo J.F.:
 Departamento de Prehistoria y Arqueología, Universidad Nacional de Educación a Distancia, Paseo Senda del Rey 7, Madrid, E-28040, Spain

West A.:
 GeoScience Consulting, Dewey, AZ 86327, United States

Kennett J.P.:
 Department of Earth Science and Marine Science Institute, University of California, Santa Barbara, CA 93106, United States

Wolbach W.S.:
 Department of Chemistry, DePaul University, Chicago, IL 60614, United States
ISSN: 00221376
Editorial
UNIV CHICAGO PRESS, 1427 E 60TH ST, CHICAGO, IL 60637-2954 USA, Estados Unidos America
Tipo de documento: Article
Volumen: 122 Número: 5
Páginas: 475-506
WOS Id: 000342508000001
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