Dependence of irradiation temperature in the response of iron salts
Por:
Martínez T., Lartigue J., Frias D., Sanchez-Mejorada G., Negrón-Mendoza A., Ramos-Bernal S.
Publicada:
1 ene 2004
Resumen:
A potential dosimeter based on aqueous frozen solutions and solid-state salt are presented for the evaluation of the energy transferred during the interaction of high-energy radiation with matter at low temperature. The foundation of these dosimeters, both the solid state and the frozen solutions, is based on the measurement of the change of the iron oxidation state. The systems were irradiated with gamma radiation at different doses (up to 10 MGy), and at different temperatures (from 77 to 298 K). The irradiated samples were analysed by UV-spectroscopy and Mössbauer spectroscopy. A theoretical model was developed for the chemical reactions system. This model reproduces the experimental effects produced by the irradiation in aqueous solutions of ferrous salt. The results showed that the response of the dosimeters depends on the irradiation temperature. At low-radiation doses, the response was linear. In particular, this work can be applied to low-temperature dosimetry can be specially applied to simulation experiments of extraterrestrial bodies, as well as in general to space research. © Published by Elsevier Ltd.
Filiaciones:
Martínez T.:
Facultad de Química, UNAM, Ciudad Universitaria, C.P. 04510, México DF, Mexico
Lartigue J.:
Facultad de Química, UNAM, Ciudad Universitaria, C.P. 04510, México DF, Mexico
Frias D.:
Depto. de Cie. Exatas e Tecnologicas, Universidad Estadual de Santa Cruz, Brazil
Sanchez-Mejorada G.:
Facultad de Medicina, UNAM, Ciudad Universitaria, C.P. 04510, México DF, Mexico
Negrón-Mendoza A.:
Instituto de Ciencias Nucleares, UNAM, A.P. 70-543, C.P. 04510, México DF, Mexico
Ramos-Bernal S.:
Instituto de Ciencias Nucleares, UNAM, A.P. 70-543, C.P. 04510, México DF, Mexico
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