Highly dispersed framework zirconium phosphates -acid catalysts for pentane and hexane isomerization


Por: Pavlova S.N., Sadykov V.A., Zabolotnaya G.V., Kochubey D.I., Maximovskaya R.I., Zaikovskii V.I., Kriventsov V.V., Tsybulya S.V., Burgina E.B., Volodin A.M., Ostrovskii N.M., Simakov A.V., Nikoro T.A., Fenelonov V.B., Chaikina M.V., Kuznetsova N.N., Lunin V.V., Agrawal D., Roy R.

Publicada: 1 ene 2000
Resumen:
The structural features, texture and surface properties of highly dispersed partially substituted framework zirconium phosphates synthesized via sol-gel or mechanochemical activation route followed by the hydrothermal treatment in the presence of polyethylene oxide were studied and compared with catalytic properties in the pentane and hexane isomerization. The most efficient promoter was found to be Si which increases the surface density of the Broensted Zr-OH centers. Pt-supported Si-modified systems demonstrate promising activity and selectivity in propane and hexane hydroisomerization at 300-400 °C. © 2000 Elsevier Science B.V. All rights reserved.

Filiaciones:
Pavlova S.N.:
 Boreskov Institute of Catalysis, SD RAN, pr. Lavrentieva, 5, 630090 Novosibirsk, Russian Federation

Sadykov V.A.:
 Boreskov Institute of Catalysis, SD RAN, pr. Lavrentieva, 5, 630090 Novosibirsk, Russian Federation

 Novosibirsk State University, Novosibirsk, Russian Federation

Zabolotnaya G.V.:
 Boreskov Institute of Catalysis, SD RAN, pr. Lavrentieva, 5, 630090 Novosibirsk, Russian Federation

Kochubey D.I.:
 Boreskov Institute of Catalysis, SD RAN, pr. Lavrentieva, 5, 630090 Novosibirsk, Russian Federation

Maximovskaya R.I.:
 Boreskov Institute of Catalysis, SD RAN, pr. Lavrentieva, 5, 630090 Novosibirsk, Russian Federation

Zaikovskii V.I.:
 Boreskov Institute of Catalysis, SD RAN, pr. Lavrentieva, 5, 630090 Novosibirsk, Russian Federation

Kriventsov V.V.:
 Boreskov Institute of Catalysis, SD RAN, pr. Lavrentieva, 5, 630090 Novosibirsk, Russian Federation

Tsybulya S.V.:
 Boreskov Institute of Catalysis, SD RAN, pr. Lavrentieva, 5, 630090 Novosibirsk, Russian Federation

Burgina E.B.:
 Boreskov Institute of Catalysis, SD RAN, pr. Lavrentieva, 5, 630090 Novosibirsk, Russian Federation

Volodin A.M.:
 Boreskov Institute of Catalysis, SD RAN, pr. Lavrentieva, 5, 630090 Novosibirsk, Russian Federation

Ostrovskii N.M.:
 Boreskov Institute of Catalysis, SD RAN, pr. Lavrentieva, 5, 630090 Novosibirsk, Russian Federation

Simakov A.V.:
 Boreskov Institute of Catalysis, SD RAN, pr. Lavrentieva, 5, 630090 Novosibirsk, Russian Federation

Nikoro T.A.:
 Boreskov Institute of Catalysis, SD RAN, pr. Lavrentieva, 5, 630090 Novosibirsk, Russian Federation

Fenelonov V.B.:
 Boreskov Institute of Catalysis, SD RAN, pr. Lavrentieva, 5, 630090 Novosibirsk, Russian Federation

Chaikina M.V.:
 Institute of Solid State Chem., Novosibirsk, Russian Federation

Kuznetsova N.N.:
 Lomonosov Moscow State University, Moscow, Russian Federation

Lunin V.V.:
 Lomonosov Moscow State University, Moscow, Russian Federation

Agrawal D.:
 Materials Research Laboratory, Pennsylvania State University, University Park, PA, United States

Roy R.:
 Materials Research Laboratory, Pennsylvania State University, University Park, PA, United States
ISSN: 01672991
Editorial
Elsevier Inc.
Tipo de documento: Article
Volumen: 130 C Número:
Páginas: 2399-2404